DG I would go for the PC version but I'm a PC gamer that has never owned a console.
You'll run into the same issues with both version...possibility of some crashes & a few other bugs. On my end the crash issues where related to audio drivers...had to revert to the oldest drivers released to be able to start the game (xonar d2x).
If you have an SLI/crossfire rig.. you should go into one of the config files in (my documents I think) & Edit to set SLI/crossfire to yes..that will eliminate the stuttering issues & improve performance. (frame rate wont drop as much).
PS. I rarely use the VATS so PC version is ideal for aiming.